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Basis sets and pseudopotentials

Which basis sets and/or pseudopotentials should I use?

When in doubt, always use the DZVP-MOLOPT-GTH basis set and the GTH-PBE pseudopotential.

  • use OT for non-metallic systems for much greater performance, with a good preconditione

Reference:

CP2k, Argone wiki
CP2k+GROMACS
CP2K
CP2K_introduction
CP2K for hybrid functionals \

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